Ruth Gordon plays Dame Marjorie 'Maude' Chardin, an eccentric and free-spirited 79-year-old woman who befriends Harold and teaches him to embrace life fully.
Bud Cort portrays Harold Parker Chasen, a young man obsessed with death who forms an unlikely bond with Maude and undergoes personal transformation.
Vivian Pickles portrays Mrs. Chasen, Harold's wealthy and overbearing mother who struggles to understand her son's unconventional behavior.
Cyril Cusack appears as Glaucus, a character in a play attended by Harold and Maude, adding to the quirky atmosphere of the film.
Charles Tyner plays Uncle Victor, a family member of Harold who disapproves of his peculiar ways and often clashes with him.
Ellen Geer portrays Sunshine Doré, a carefree and nature-loving young woman who briefly enters Harold's life.
Eric Christmas appears as the Priest who officiates a scene in the film, providing a traditional contrast to the unconventional nature of Harold and Maude's relationship.
G. Wood plays the Psychiatrist who treats Harold, offering a professional perspective on his behavior and mindset.
Judy Engles portrays Candy Gulf, a character in a play attended by Harold and Maude, adding to the whimsical nature of the film.
Shari Summers plays Edith Phern, a character in a play attended by Harold and Maude, contributing to the film's eclectic and eccentric atmosphere.
Tom Skerritt appears as the Motorcycle Officer who has a brief encounter with Harold and Maude during one of their escapades.
Susan Madigan portrays Girlfriend, a brief romantic interest of Harold who struggles to understand his unusual preferences and behavior.
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