Arnold Stang voices Top Cat, the charismatic and quick-witted alley cat who leads his gang on various schemes.
Avery Schreiber provides the voice for Benny the Ball, the loyal and somewhat slow-witted member of Top Cat's gang.
Kenneth Mars lends his voice to the characters of Director and Dogcatcher in the movie.
Rob Paulsen voices James the Chauffeur, Lester Pester, and the Tour Bus Driver, adding humor and versatility to the characters.
Richard Erdman voices Sid Buckman and the Car Wash Manager, portraying a variety of roles in the film.
John Stephenson provides the voices for Fancy-Fancy, Officer Charlie Dibble, and the Waiter, adding depth to each character.
Marvin Kaplan voices Choo-Choo, one of the loyal members of Top Cat's gang.
Henry Polic II voices Snerdly, adding his unique touch to the character.
Lilly Moon gives her voice to the character of Amy Vandergelt in the movie.
Teresa Ganzel voices Kitty Glitter, adding flair to the glamorous character in the film.
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