Faye Dunaway portrays Lady Barbara Skelton, a noblewoman who leads a double life as a highwaywoman in The Wicked Lady.
Alan Bates plays Captain Jerry Jackson, a charming highwayman who becomes romantically involved with Lady Barbara Skelton.
John Gielgud takes on the role of Hogarth, an elderly servant who is loyal to Lady Barbara Skelton throughout her adventures.
Denholm Elliott portrays Sir Ralph Skelton, Lady Barbara's husband who becomes a target of her criminal activities.
Prunella Scales plays Lady Kingsclere, a member of high society who is acquainted with Lady Barbara Skelton.
Oliver Tobias is Kit Locksby, a gentleman who is romantically linked to Lady Barbara Skelton before her descent into crime.
Glynis Barber portrays Caroline, a supportive friend of Lady Barbara Skelton who gets entangled in her illicit activities.
Joan Hickson takes on the role of Aunt Agatha, a family member of Lady Barbara Skelton who disapproves of her behavior.
Helena McCarthy plays Moll Skelton, a relative of Lady Barbara Skelton who is impacted by her criminal deeds.
Mollie Maureen portrays Doll Skelton, another family member of Lady Barbara Skelton who experiences the consequences of her actions.
Derek Francis is Lord Kingsclere, a wealthy nobleman who is connected to the social circle of Lady Barbara Skelton.
Marina Sirtis appears as Jackson's Girl, a character linked to Captain Jerry Jackson who becomes involved in the intrigue surrounding Lady Barbara Skelton.
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